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I am afraid to answer, because this is obviously impossible to answer based on facts... Personally I would recommend to pick movies according to your most liked genres first as they might keep you interested the most. It's probably near to impossible to suggest movies from one's own likings. But since you've asked - go for "Das Experiment", "Das Boot", ...
I saw recently a movie called "Wo ist Fred?". There are pretty simple word-stock and the good actors such as Til Schweiger.
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